Annihilation of the triplet excitons in the nanoporous glass matrices

dc.contributor.authorAfanasyev, D.A.
dc.contributor.authorIbrayev, N.Kh.
dc.contributor.authorSaletsky, A.M.
dc.contributor.authorStarokurov, Y.V.
dc.contributor.authorGun’ko, V.M.
dc.contributor.authorMikhalovsky, S.V.
dc.date.accessioned2017-01-10T05:31:32Z
dc.date.available2017-01-10T05:31:32Z
dc.date.issued2013-04
dc.description.abstractThe spectraandkineticsoffluorescencedecayof1,2-benzanthracene(1,2-BA)molecularclusters adsorbedinnanoporousborosilicateglasseswereinvestigated.Ithasbeenshownthatthetypeofthe decaykineticsofdelayedfluorescenceisdeterminedbytheannihilationoftripletexcitonsincrystalline andpercolationclusters.Theinfluenceofanexternalmagneticfieldontheannihilationrateconstantof tripletexcitonsintheadsorbed1,2-BAmoleculeshasbeenstudied.Theresponseofthemolecular clusterstothemagneticfieldstronglydependsontemperature,poresizeandtimescaleofthe observation.Clusterswiththecrystalstructuredominateinthedecaykineticsoftriplet–triplet annihilation(TTA)anddelayedfluorescenceintheinitialmicrosecondperiodoftimeafterexcitation. Amorphousclustersdeterminetheformofdecaykineticsofdelayedfluorescenceinthemillisecond range.Theincreaseintheporesizeandconcentrationoftheadsorbateleadtothedominanceof crystallinecomponents.Theresultspresentedherecanbeusedtodeveloptechniquesforprobingthe structureoftheadsorbedlayerinnanoporoussystemsexaminingtheeffectofanexternalmagneticfield on theannihilationdelayedfluorescence(ADF)kinetics.ru_RU
dc.identifier.citationAnnihilation of the triplet excitons in the nanoporous glass matrices / D. A. Afanasyev[a.o.]//Journal ofLuminescence. - Amsterdam: Elsevier science bv. - 2013. - Vol.136. - p.358-364. - ISSN 0022-2313
dc.identifier.issn0022-2313
dc.identifier.urihttps://rep.buketov.edu.kz/handle/data/646
dc.language.isoenru_RU
dc.publisherElsevier science bvru_RU
dc.relation.ispartofseriesJournal ofLuminescence;Vol.136.
dc.subjectDelayed fluorescenceru_RU
dc.subjectTriplet–triplet annihilationru_RU
dc.subjectMagnetic fieldeffectru_RU
dc.subjectPorous glassesru_RU
dc.subjectMolecular clustersru_RU
dc.titleAnnihilation of the triplet excitons in the nanoporous glass matricesru_RU
dc.typeArticleru_RU

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